Two-dimensional electronic spectroscopy for mapping molecular photophysics

Jessica M. Anna; Yin Song; Rayomond Dinshaw; Gregory D. Scholes

doi:10.1351/PAC-CON-12-10-21

Two-dimensional electronic spectroscopy for mapping molecular photophysics

Jessica M. Anna, Yin Song, Rayomond Dinshaw, Gregory D. Scholes

Research output: Contribution to journal › Article › peer-review

26 Scopus citations

Abstract

We demonstrate the ability of two-dimensional electronic spectroscopy (2DES) to map ultrafast energy transfer and dynamics in two systems: the pigment-protein complex photosystem I (PSI) and aggregates of the conjugated polymer poly(3-hexylthiophene) (P3HT). A detailed description of our experimental set-up and data processing procedure is also given.

Original language	English (US)
Pages (from-to)	1307-1319
Number of pages	13
Journal	Pure and Applied Chemistry
Volume	85
Issue number	7
DOIs	https://doi.org/10.1351/PAC-CON-12-10-21
State	Published - 2013
Externally published	Yes

All Science Journal Classification (ASJC) codes

General Chemistry
General Chemical Engineering

Keywords

Energy transfer
Light harvesting
Molecular aggregates
Phasing
Photosynthesis
Two-dimensional electronic spectroscopy
Ultrafast spectroscopy

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10.1351/PAC-CON-12-10-21

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title = "Two-dimensional electronic spectroscopy for mapping molecular photophysics",

abstract = "We demonstrate the ability of two-dimensional electronic spectroscopy (2DES) to map ultrafast energy transfer and dynamics in two systems: the pigment-protein complex photosystem I (PSI) and aggregates of the conjugated polymer poly(3-hexylthiophene) (P3HT). A detailed description of our experimental set-up and data processing procedure is also given.",

keywords = "Energy transfer, Light harvesting, Molecular aggregates, Phasing, Photosynthesis, Two-dimensional electronic spectroscopy, Ultrafast spectroscopy",

author = "Anna, {Jessica M.} and Yin Song and Rayomond Dinshaw and Scholes, {Gregory D.}",

note = "Funding Information: This work was supported by DARPA under the QuBE program, the United States Air Force Office of Scientific Research (FA9550-10-1-0260), and the Natural Sciences and Engineering Research Council of Canada",

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doi = "10.1351/PAC-CON-12-10-21",

language = "English (US)",

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pages = "1307--1319",

journal = "Pure and Applied Chemistry",

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TY - JOUR

T1 - Two-dimensional electronic spectroscopy for mapping molecular photophysics

AU - Anna, Jessica M.

AU - Song, Yin

AU - Dinshaw, Rayomond

AU - Scholes, Gregory D.

N1 - Funding Information: This work was supported by DARPA under the QuBE program, the United States Air Force Office of Scientific Research (FA9550-10-1-0260), and the Natural Sciences and Engineering Research Council of Canada

PY - 2013

Y1 - 2013

N2 - We demonstrate the ability of two-dimensional electronic spectroscopy (2DES) to map ultrafast energy transfer and dynamics in two systems: the pigment-protein complex photosystem I (PSI) and aggregates of the conjugated polymer poly(3-hexylthiophene) (P3HT). A detailed description of our experimental set-up and data processing procedure is also given.

AB - We demonstrate the ability of two-dimensional electronic spectroscopy (2DES) to map ultrafast energy transfer and dynamics in two systems: the pigment-protein complex photosystem I (PSI) and aggregates of the conjugated polymer poly(3-hexylthiophene) (P3HT). A detailed description of our experimental set-up and data processing procedure is also given.

KW - Energy transfer

KW - Light harvesting

KW - Molecular aggregates

KW - Phasing

KW - Photosynthesis

KW - Two-dimensional electronic spectroscopy

KW - Ultrafast spectroscopy

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DO - 10.1351/PAC-CON-12-10-21

M3 - Article

AN - SCOPUS:84880083249

SN - 0033-4545

VL - 85

SP - 1307

EP - 1319

JO - Pure and Applied Chemistry

JF - Pure and Applied Chemistry

IS - 7

ER -

Two-dimensional electronic spectroscopy for mapping molecular photophysics

Abstract

All Science Journal Classification (ASJC) codes

Keywords

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