Tropical dehydration processes constrained by the seasonality of stratospheric deuterated water

Jörg Steinwagner, Stephan Andreas Fueglistaler, Gabriele Stiller, Thomas Von Clarmann, Michael Kiefer, Peter Paul Borsboom, Aarnout Van Delden, Thomas Röckmann

Research output: Contribution to journalArticle

41 Scopus citations

Abstract

Stratospheric water vapour affects Earths radiation budget. In addition, it has a key role in stratospheric chemistry and in processes that permit ozone depletion. Air largely enters the stratosphere in the tropics, but the processes that bring water through the cold tropopause into the stratosphere are not well understood. Here we present a 19-month record of non-deuterated (H 2O) and deuterated (HDO) water in the tropical stratosphere, collected through remote-sensing measurements with the Michelson Interferometer for Passive Atmospheric Sounding. Our data show a clear seasonal cycle in the isotopic composition that propagates upward in the tropical stratosphere, and is most likely created in the tropical tropopause layer. In addition, we find that the slope of the HDO-H 2 O correlation of water entering the stratosphere in the tropics is close to, but slightly steeper than the slope expected from Rayleigh fractionation. We propose that gradual dehydration of air by cirrus clouds that are formed in situ, together with a seasonally varying contribution from the evaporation of convectively lofted ice, provides the most plausible explanation for our measurements. We conclude that potential changes in the water budget of the tropical tropopause layer and the stratosphere should be detectable in isotopic measurements.

Original languageEnglish (US)
Pages (from-to)262-266
Number of pages5
JournalNature Geoscience
Volume3
Issue number4
DOIs
StatePublished - Apr 1 2010

All Science Journal Classification (ASJC) codes

  • Earth and Planetary Sciences(all)

Fingerprint Dive into the research topics of 'Tropical dehydration processes constrained by the seasonality of stratospheric deuterated water'. Together they form a unique fingerprint.

  • Cite this

    Steinwagner, J., Fueglistaler, S. A., Stiller, G., Von Clarmann, T., Kiefer, M., Borsboom, P. P., Van Delden, A., & Röckmann, T. (2010). Tropical dehydration processes constrained by the seasonality of stratospheric deuterated water. Nature Geoscience, 3(4), 262-266. https://doi.org/10.1038/ngeo822