Theoretical prediction of the effective dynamic dielectric constant of disordered hyperuniform anisotropic composites beyond the long-wavelength regime [Invited]

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Abstract

Torquato and Kim [Phys. Rev. X 11, 296 021002 (2021)] derived exact nonlocal strong-contrast expansions of the effective dynamic dielectric constant tensor εe(kq, ω) that treat general statistically anisoropic three-dimensional (3D) two-phase composite microstructures, which are valid well beyond the long-wavelength regime. Here, we demonstrate that truncating this general rapidly converging expansion at the two- and three-point levels is a powerful theoretical tool from which one can extract accurate approximations suited for various microstructural symmetries. Among other results, we show that such truncations yield closed-form formulas applicable to transverse polarization in layered media and transverse magnetic polarization in transversely isotropic media, respectively. We apply these formulas to estimate εe(kq, ω) for models of 3D disordered hyperuniform layered and transversely isotropic media: nonstealthy hyperuniform media and stealthy hyperuniform media. In particular, we show that stealthy hyperuniform layered and transversely isotropic media are perfectly transparent (trivially implying no Anderson localization, in principle) within finite wave number intervals through the third-order terms. For all models considered here, we validate that the second-order formulas, which depend on the spectral density, are already very accurate well beyond the long-wavelength regime by showing very good agreement with the finite-difference time-domain (FDTD) simulations. The high predictive power of the second-order formula is due to the fact that higher-order contributions are negligibly small, implying that it very accurately approximates multiple scattering through all orders. This implies that there can be no Anderson localization within the predicted perfect transparency interval in stealthy hyperuniform layered and transversely isotropic media in practice because the localization length (associated with only possibly negligibly small higher-order contributions) should be very large compared to any practically large sample size. Our predictive theory provides the foundation for the inverse design of novel effective wave characteristics of disordered and statistically anisotropic structures by engineering their spectral densities.

Original languageEnglish (US)
Pages (from-to)194-215
Number of pages22
JournalOptical Materials Express
Volume14
Issue number1
DOIs
StatePublished - Jan 2024

All Science Journal Classification (ASJC) codes

  • Electronic, Optical and Magnetic Materials

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