TY - JOUR
T1 - The properties and prospects of chemically exfoliated nanosheets for quantum materials in two dimensions
AU - Song, Xiaoyu
AU - Yuan, Fang
AU - Schoop, Leslie M.
N1 - Funding Information:
This work was supported by the Princeton Center for Complex Materials, a National Science Foundation (NSF)-MRSEC program (DMR-2011750), the Gordon and Betty Moore Foundation (Grant No. GBMF9064), and the Princeton Catalysis Initiative (PCI). The authors acknowledge Dr. Guangming Chen and Dr. Nan Yao at the Imaging Analysis Center of Princeton Institute for the Science and Technology of Materials in assisting us in acquiring the images shown in Fig. 23. The authors acknowledge the use of Princeton’s Imaging and Analysis Center, which is partially supported by the NSF-MRSEC program, above.
Publisher Copyright:
© 2021 Author(s).
PY - 2021/3/1
Y1 - 2021/3/1
N2 - The aim of this review is to elucidate the potential of chemically exfoliated sheets for the field of quantum matter. Quantum materials are loosely defined as materials that do not follow the laws of classical physics; the family commonly includes complex magnets, topological materials, or superconductors. Two-dimensional (2D) materials have been key in driving the field of quantum matter forward due to the high degree of tunability they offer. However, progress has largely been made with mechanically exfoliated sheets while chemically exfoliated sheets have been mostly ignored. The latter offer a wide range of advantages, for example, chemical exfoliation gives access to 2D materials that are unobtainable with other methods. In this review, we highlight the progress that has been made in exploring properties that can be associated with quantum materials of chemically exfoliated nanosheets. We will cover magnetic chemically exfoliated sheets, their use in transistors, their potential as 2D topological insulators, and opportunities that arise for the emerging field of twistronics. We will highlight both the advantages and current shortcomings of chemically exfoliated quantum materials and address how shortcomings might be overcome in the future. We conclude that while the prospects of chemically exfoliated sheets for quantum materials are still underexplored, they offer a large potential for having an impact in that field.
AB - The aim of this review is to elucidate the potential of chemically exfoliated sheets for the field of quantum matter. Quantum materials are loosely defined as materials that do not follow the laws of classical physics; the family commonly includes complex magnets, topological materials, or superconductors. Two-dimensional (2D) materials have been key in driving the field of quantum matter forward due to the high degree of tunability they offer. However, progress has largely been made with mechanically exfoliated sheets while chemically exfoliated sheets have been mostly ignored. The latter offer a wide range of advantages, for example, chemical exfoliation gives access to 2D materials that are unobtainable with other methods. In this review, we highlight the progress that has been made in exploring properties that can be associated with quantum materials of chemically exfoliated nanosheets. We will cover magnetic chemically exfoliated sheets, their use in transistors, their potential as 2D topological insulators, and opportunities that arise for the emerging field of twistronics. We will highlight both the advantages and current shortcomings of chemically exfoliated quantum materials and address how shortcomings might be overcome in the future. We conclude that while the prospects of chemically exfoliated sheets for quantum materials are still underexplored, they offer a large potential for having an impact in that field.
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U2 - 10.1063/5.0038644
DO - 10.1063/5.0038644
M3 - Review article
AN - SCOPUS:85103633692
SN - 1931-9401
VL - 8
JO - Applied Physics Reviews
JF - Applied Physics Reviews
IS - 1
M1 - 011312
ER -