The declining uptake rate of atmospheric CO2 by land and ocean sinks

M. R. Raupach, M. Gloor, Jorge Louis Sarmiento, J. G. Canadell, T. L. Frölicher, T. Gasser, R. A. Houghton, C. Le Quéré, C. M. Trudinger

Research output: Contribution to journalArticlepeer-review

61 Scopus citations


Through 1959-2012, an airborne fraction (AF) of 0.44 of total anthropogenic CO2 emissions remained in the atmosphere, with the rest being taken up by land and ocean CO2 sinks. Understanding of this uptake is critical because it greatly alleviates the emissions reductions required for climate mitigation, and also reduces the risks and damages that adaptation has to embrace. An observable quantity that reflects sink properties more directly than the AF is the CO 2 sink rate (kS), the combined land-ocean CO2 sink flux per unit excess atmospheric CO2 above preindustrial levels. Here we show from observations thatkS declined over 1959-2012 by a factor of about 1 / 3, implying that CO2 sinks increased more slowly than excess CO2. Using a carbon-climate model, we attribute the decline inkS to four mechanisms: slower-than-exponential CO2 emissions growth (∼ 35% of the trend), volcanic eruptions (∼ 25%), sink responses to climate change (∼ 20%), and nonlinear responses to increasing CO2, mainly oceanic (∼ 20%). The first of these mechanisms is associated purely with the trajectory of extrinsic forcing, and the last two with intrinsic, feedback responses of sink processes to changes in climate and atmospheric CO2. Our results suggest that the effects of these intrinsic, nonlinear responses are already detectable in the global carbon cycle. Although continuing future decreases inkS will occur under all plausible CO2 emission scenarios, the rate of decline varies between scenarios in non-intuitive ways because extrinsic and intrinsic mechanisms respond in opposite ways to changes in emissions: extrinsic mechanisms causekS to decline more strongly with increasing mitigation, while intrinsic mechanisms causekS to decline more strongly under high-emission, low-mitigation scenarios as the carbon-climate system is perturbed further from a near-linear regime.

Original languageEnglish (US)
Pages (from-to)3453-3475
Number of pages23
Issue number13
StatePublished - Jul 2 2014

All Science Journal Classification (ASJC) codes

  • Ecology, Evolution, Behavior and Systematics
  • Earth-Surface Processes


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