TY - JOUR
T1 - Selective excitation of molecular eigenstates using state-dependent optical field design
AU - Chen, Yu
AU - Gross, Peter
AU - Ramakrishna, Viswanath
AU - Rabitz, Herschel
AU - Mease, Kenneth
N1 - Funding Information:
We acknowledge support for this research from the Office of Naval Research and the Army Research Office.
Copyright:
Copyright 2020 Elsevier B.V., All rights reserved.
PY - 1996/4/19
Y1 - 1996/4/19
N2 - A new feedback algorithm to design laser fields for state-selective excitation of molecular systems is proposed. The population amplitudes and relative phases of the eigenstates are used to generate a field which drives the population flow in the desired direction. Results are presented for both vibrational excitation of hydrogen fluoride and selective excitation of one of two degenerate electronic states in a model four level system.
AB - A new feedback algorithm to design laser fields for state-selective excitation of molecular systems is proposed. The population amplitudes and relative phases of the eigenstates are used to generate a field which drives the population flow in the desired direction. Results are presented for both vibrational excitation of hydrogen fluoride and selective excitation of one of two degenerate electronic states in a model four level system.
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U2 - 10.1016/0009-2614(96)00200-x
DO - 10.1016/0009-2614(96)00200-x
M3 - Article
AN - SCOPUS:0030593170
VL - 252
SP - 447
EP - 456
JO - Chemical Physics Letters
JF - Chemical Physics Letters
SN - 0009-2614
IS - 5-6
ER -