Selective excitation of molecular eigenstates using state-dependent optical field design

Yu Chen; Peter Gross; Viswanath Ramakrishna; Herschel Rabitz; Kenneth Mease

doi:10.1016/0009-2614(96)00200-x

Selective excitation of molecular eigenstates using state-dependent optical field design

Yu Chen, Peter Gross, Viswanath Ramakrishna, Herschel Rabitz, Kenneth Mease

Research output: Contribution to journal › Article › peer-review

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Abstract

A new feedback algorithm to design laser fields for state-selective excitation of molecular systems is proposed. The population amplitudes and relative phases of the eigenstates are used to generate a field which drives the population flow in the desired direction. Results are presented for both vibrational excitation of hydrogen fluoride and selective excitation of one of two degenerate electronic states in a model four level system.

Original language	English (US)
Pages (from-to)	447-456
Number of pages	10
Journal	Chemical Physics Letters
Volume	252
Issue number	5-6
DOIs	https://doi.org/10.1016/0009-2614(96)00200-x
State	Published - Apr 19 1996

All Science Journal Classification (ASJC) codes

General Physics and Astronomy
Physical and Theoretical Chemistry

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10.1016/0009-2614(96)00200-x

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title = "Selective excitation of molecular eigenstates using state-dependent optical field design",

abstract = "A new feedback algorithm to design laser fields for state-selective excitation of molecular systems is proposed. The population amplitudes and relative phases of the eigenstates are used to generate a field which drives the population flow in the desired direction. Results are presented for both vibrational excitation of hydrogen fluoride and selective excitation of one of two degenerate electronic states in a model four level system.",

author = "Yu Chen and Peter Gross and Viswanath Ramakrishna and Herschel Rabitz and Kenneth Mease",

year = "1996",

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doi = "10.1016/0009-2614(96)00200-x",

language = "English (US)",

volume = "252",

pages = "447--456",

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T1 - Selective excitation of molecular eigenstates using state-dependent optical field design

AU - Chen, Yu

AU - Gross, Peter

AU - Ramakrishna, Viswanath

AU - Rabitz, Herschel

AU - Mease, Kenneth

PY - 1996/4/19

Y1 - 1996/4/19

N2 - A new feedback algorithm to design laser fields for state-selective excitation of molecular systems is proposed. The population amplitudes and relative phases of the eigenstates are used to generate a field which drives the population flow in the desired direction. Results are presented for both vibrational excitation of hydrogen fluoride and selective excitation of one of two degenerate electronic states in a model four level system.

AB - A new feedback algorithm to design laser fields for state-selective excitation of molecular systems is proposed. The population amplitudes and relative phases of the eigenstates are used to generate a field which drives the population flow in the desired direction. Results are presented for both vibrational excitation of hydrogen fluoride and selective excitation of one of two degenerate electronic states in a model four level system.

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UR - http://www.scopus.com/inward/citedby.url?scp=0030593170&partnerID=8YFLogxK

U2 - 10.1016/0009-2614(96)00200-x

DO - 10.1016/0009-2614(96)00200-x

M3 - Article

AN - SCOPUS:0030593170

SN - 0009-2614

VL - 252

SP - 447

EP - 456

JO - Chemical Physics Letters

JF - Chemical Physics Letters

IS - 5-6

ER -

Selective excitation of molecular eigenstates using state-dependent optical field design

Abstract

All Science Journal Classification (ASJC) codes

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