Response to Comment on “Quantifying hot carrier and thermal contributions in plasmonic photocatalysis”

Linan Zhou; Dayne F. Swearer; Hossein Robatjazi; Alessandro Alabastri; Phillip Christopher; Emily Ann Carter; Peter Nordlander; Naomi J. Halas

doi:10.1126/science.aaw9545

Response to Comment on “Quantifying hot carrier and thermal contributions in plasmonic photocatalysis”

Linan Zhou, Dayne F. Swearer, Hossein Robatjazi, Alessandro Alabastri, Phillip Christopher, Emily Ann Carter, Peter Nordlander, Naomi J. Halas

Research output: Contribution to journal › Review article › peer-review

56 Scopus citations

Abstract

Sivan et al. claim that the methods used to distinguish thermal from hot carrier effects in our recent report are inaccurate and that our data can be explained by a purely thermal mechanism with a fixed activation energy. This conclusion is invalid, because they substantially misinterpret the emissivity of the photocatalyst and assume a linear intensity–dependent temperature in their model that is unrealistic.

Original language	English (US)
Article number	eaaw9545
Journal	Science
Volume	364
Issue number	6439
DOIs	https://doi.org/10.1126/science.aaw9545
State	Published - May 3 2019

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title = "Response to Comment on “Quantifying hot carrier and thermal contributions in plasmonic photocatalysis”",

abstract = "Sivan et al. claim that the methods used to distinguish thermal from hot carrier effects in our recent report are inaccurate and that our data can be explained by a purely thermal mechanism with a fixed activation energy. This conclusion is invalid, because they substantially misinterpret the emissivity of the photocatalyst and assume a linear intensity–dependent temperature in their model that is unrealistic.",

author = "Linan Zhou and Swearer, {Dayne F.} and Hossein Robatjazi and Alessandro Alabastri and Phillip Christopher and Carter, {Emily Ann} and Peter Nordlander and Halas, {Naomi J.}",

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AU - Zhou, Linan

AU - Swearer, Dayne F.

AU - Robatjazi, Hossein

AU - Alabastri, Alessandro

AU - Christopher, Phillip

AU - Carter, Emily Ann

AU - Nordlander, Peter

AU - Halas, Naomi J.

PY - 2019/5/3

Y1 - 2019/5/3

N2 - Sivan et al. claim that the methods used to distinguish thermal from hot carrier effects in our recent report are inaccurate and that our data can be explained by a purely thermal mechanism with a fixed activation energy. This conclusion is invalid, because they substantially misinterpret the emissivity of the photocatalyst and assume a linear intensity–dependent temperature in their model that is unrealistic.

AB - Sivan et al. claim that the methods used to distinguish thermal from hot carrier effects in our recent report are inaccurate and that our data can be explained by a purely thermal mechanism with a fixed activation energy. This conclusion is invalid, because they substantially misinterpret the emissivity of the photocatalyst and assume a linear intensity–dependent temperature in their model that is unrealistic.

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Response to Comment on “Quantifying hot carrier and thermal contributions in plasmonic photocatalysis”

Abstract

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