TY - JOUR
T1 - Quantum textures of the many-body wavefunctions in magic-angle graphene
AU - Nuckolls, Kevin P.
AU - Lee, Ryan L.
AU - Oh, Myungchul
AU - Wong, Dillon
AU - Soejima, Tomohiro
AU - Hong, Jung Pyo
AU - Călugăru, Dumitru
AU - Herzog-Arbeitman, Jonah
AU - Bernevig, B. Andrei
AU - Watanabe, Kenji
AU - Taniguchi, Takashi
AU - Regnault, Nicolas
AU - Zaletel, Michael P.
AU - Yazdani, Ali
N1 - Publisher Copyright:
© 2023, The Author(s), under exclusive licence to Springer Nature Limited.
PY - 2023/8/17
Y1 - 2023/8/17
N2 - Interactions among electrons create novel many-body quantum phases of matter with wavefunctions that reflect electronic correlation effects, broken symmetries and collective excitations. Many quantum phases have been discovered in magic-angle twisted bilayer graphene (MATBG), including correlated insulating1, unconventional superconducting2–5 and magnetic topological6–9 phases. The lack of microscopic information10,11 of possible broken symmetries has hampered our understanding of these phases12–17. Here we use high-resolution scanning tunnelling microscopy to study the wavefunctions of the correlated phases in MATBG. The squares of the wavefunctions of gapped phases, including those of the correlated insulating, pseudogap and superconducting phases, show distinct broken-symmetry patterns with a √3 × √3 super-periodicity on the graphene atomic lattice that has a complex spatial dependence on the moiré scale. We introduce a symmetry-based analysis using a set of complex-valued local order parameters, which show intricate textures that distinguish the various correlated phases. We compare the observed quantum textures of the correlated insulators at fillings of ±2 electrons per moiré unit cell to those expected for proposed theoretical ground states. In typical MATBG devices, these textures closely match those of the proposed incommensurate Kekulé spiral order15, whereas in ultralow-strain samples, our data have local symmetries like those of a time-reversal symmetric intervalley coherent phase12. Moreover, the superconducting state of MATBG shows strong signatures of intervalley coherence, only distinguishable from those of the insulator with our phase-sensitive measurements.
AB - Interactions among electrons create novel many-body quantum phases of matter with wavefunctions that reflect electronic correlation effects, broken symmetries and collective excitations. Many quantum phases have been discovered in magic-angle twisted bilayer graphene (MATBG), including correlated insulating1, unconventional superconducting2–5 and magnetic topological6–9 phases. The lack of microscopic information10,11 of possible broken symmetries has hampered our understanding of these phases12–17. Here we use high-resolution scanning tunnelling microscopy to study the wavefunctions of the correlated phases in MATBG. The squares of the wavefunctions of gapped phases, including those of the correlated insulating, pseudogap and superconducting phases, show distinct broken-symmetry patterns with a √3 × √3 super-periodicity on the graphene atomic lattice that has a complex spatial dependence on the moiré scale. We introduce a symmetry-based analysis using a set of complex-valued local order parameters, which show intricate textures that distinguish the various correlated phases. We compare the observed quantum textures of the correlated insulators at fillings of ±2 electrons per moiré unit cell to those expected for proposed theoretical ground states. In typical MATBG devices, these textures closely match those of the proposed incommensurate Kekulé spiral order15, whereas in ultralow-strain samples, our data have local symmetries like those of a time-reversal symmetric intervalley coherent phase12. Moreover, the superconducting state of MATBG shows strong signatures of intervalley coherence, only distinguishable from those of the insulator with our phase-sensitive measurements.
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U2 - 10.1038/s41586-023-06226-x
DO - 10.1038/s41586-023-06226-x
M3 - Article
C2 - 37587297
AN - SCOPUS:85168240026
SN - 0028-0836
VL - 620
SP - 525
EP - 532
JO - Nature
JF - Nature
IS - 7974
ER -