TY - JOUR
T1 - Quantum textures of the many-body wavefunctions in magic-angle graphene
AU - Nuckolls, Kevin P.
AU - Lee, Ryan L.
AU - Oh, Myungchul
AU - Wong, Dillon
AU - Soejima, Tomohiro
AU - Hong, Jung Pyo
AU - Călugăru, Dumitru
AU - Herzog-Arbeitman, Jonah
AU - Bernevig, B. Andrei
AU - Watanabe, Kenji
AU - Taniguchi, Takashi
AU - Regnault, Nicolas
AU - Zaletel, Michael P.
AU - Yazdani, Ali
N1 - Funding Information:
We thank O. Vafek, X. Liu, C.-L. Chiu and G. Farahi for discussions; and H. Ding for technical discussion. This work was primarily supported by the Gordon and Betty Moore Foundation’s EPiQS initiative grants GBMF9469 and DOE-BES grant DE-FG02-07ER46419 to A.Y. Other support for the experimental work was provided by NSF-MRSEC through the Princeton Center for Complex Materials NSF-DMR- 2011750, NSF-DMR-1904442, ARO MURI (W911NF-21-2-0147) and ONR N00012-21-1-2592. T.S. was supported by a fellowship from the Masason Foundation, and by the US Department of Energy, Office of Science, National Quantum Information Science Research Centers, Quantum Systems Accelerator. J.P.H. was supported by the Princeton University Department of Physics. M.P.Z. was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under contract no. DE-AC02-05CH11231, within the van der Waals Heterostructures Program (KCWF16), and the Alfred P. Sloan Foundation. D.C., B.A.B. and N.R. were supported by the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation programme (grant agreement no. 101020833), the ONR grant no. N00014-20-1-2303, Simons Investigator grant no. 404513, the Gordon and Betty Moore Foundation through the EPiQS Initiative, grant no. GBMF11070 and grant no. GBMF8685, NSF-MRSEC grant no. DMR-2011750, BSF Israel US foundation grant no. 2018226, and the Princeton Global Network Funds. J.H.-A. was supported by a Hertz Fellowship. N.R. acknowledges support from the QuantERA II Programme that has received funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement no. 101017733. K.W. and T.T. acknowledge support from the Elemental Strategy Initiative conducted by the MEXT, Japan, grant JPMXP0112101001, JSPS KAKENHI grants 19H05790 and JP20H00354.
Funding Information:
We thank O. Vafek, X. Liu, C.-L. Chiu and G. Farahi for discussions; and H. Ding for technical discussion. This work was primarily supported by the Gordon and Betty Moore Foundation’s EPiQS initiative grants GBMF9469 and DOE-BES grant DE-FG02-07ER46419 to A.Y. Other support for the experimental work was provided by NSF-MRSEC through the Princeton Center for Complex Materials NSF-DMR- 2011750, NSF-DMR-1904442, ARO MURI (W911NF-21-2-0147) and ONR N00012-21-1-2592. T.S. was supported by a fellowship from the Masason Foundation, and by the US Department of Energy, Office of Science, National Quantum Information Science Research Centers, Quantum Systems Accelerator. J.P.H. was supported by the Princeton University Department of Physics. M.P.Z. was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under contract no. DE-AC02-05CH11231, within the van der Waals Heterostructures Program (KCWF16), and the Alfred P. Sloan Foundation. D.C., B.A.B. and N.R. were supported by the European Research Council (ERC) under the European Union’s Horizon 2020 research and innovation programme (grant agreement no. 101020833), the ONR grant no. N00014-20-1-2303, Simons Investigator grant no. 404513, the Gordon and Betty Moore Foundation through the EPiQS Initiative, grant no. GBMF11070 and grant no. GBMF8685, NSF-MRSEC grant no. DMR-2011750, BSF Israel US foundation grant no. 2018226, and the Princeton Global Network Funds. J.H.-A. was supported by a Hertz Fellowship. N.R. acknowledges support from the QuantERA II Programme that has received funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement no. 101017733. K.W. and T.T. acknowledge support from the Elemental Strategy Initiative conducted by the MEXT, Japan, grant JPMXP0112101001, JSPS KAKENHI grants 19H05790 and JP20H00354.
Publisher Copyright:
© 2023, The Author(s), under exclusive licence to Springer Nature Limited.
PY - 2023/8/17
Y1 - 2023/8/17
N2 - Interactions among electrons create novel many-body quantum phases of matter with wavefunctions that reflect electronic correlation effects, broken symmetries and collective excitations. Many quantum phases have been discovered in magic-angle twisted bilayer graphene (MATBG), including correlated insulating1, unconventional superconducting2–5 and magnetic topological6–9 phases. The lack of microscopic information10,11 of possible broken symmetries has hampered our understanding of these phases12–17. Here we use high-resolution scanning tunnelling microscopy to study the wavefunctions of the correlated phases in MATBG. The squares of the wavefunctions of gapped phases, including those of the correlated insulating, pseudogap and superconducting phases, show distinct broken-symmetry patterns with a √3 × √3 super-periodicity on the graphene atomic lattice that has a complex spatial dependence on the moiré scale. We introduce a symmetry-based analysis using a set of complex-valued local order parameters, which show intricate textures that distinguish the various correlated phases. We compare the observed quantum textures of the correlated insulators at fillings of ±2 electrons per moiré unit cell to those expected for proposed theoretical ground states. In typical MATBG devices, these textures closely match those of the proposed incommensurate Kekulé spiral order15, whereas in ultralow-strain samples, our data have local symmetries like those of a time-reversal symmetric intervalley coherent phase12. Moreover, the superconducting state of MATBG shows strong signatures of intervalley coherence, only distinguishable from those of the insulator with our phase-sensitive measurements.
AB - Interactions among electrons create novel many-body quantum phases of matter with wavefunctions that reflect electronic correlation effects, broken symmetries and collective excitations. Many quantum phases have been discovered in magic-angle twisted bilayer graphene (MATBG), including correlated insulating1, unconventional superconducting2–5 and magnetic topological6–9 phases. The lack of microscopic information10,11 of possible broken symmetries has hampered our understanding of these phases12–17. Here we use high-resolution scanning tunnelling microscopy to study the wavefunctions of the correlated phases in MATBG. The squares of the wavefunctions of gapped phases, including those of the correlated insulating, pseudogap and superconducting phases, show distinct broken-symmetry patterns with a √3 × √3 super-periodicity on the graphene atomic lattice that has a complex spatial dependence on the moiré scale. We introduce a symmetry-based analysis using a set of complex-valued local order parameters, which show intricate textures that distinguish the various correlated phases. We compare the observed quantum textures of the correlated insulators at fillings of ±2 electrons per moiré unit cell to those expected for proposed theoretical ground states. In typical MATBG devices, these textures closely match those of the proposed incommensurate Kekulé spiral order15, whereas in ultralow-strain samples, our data have local symmetries like those of a time-reversal symmetric intervalley coherent phase12. Moreover, the superconducting state of MATBG shows strong signatures of intervalley coherence, only distinguishable from those of the insulator with our phase-sensitive measurements.
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U2 - 10.1038/s41586-023-06226-x
DO - 10.1038/s41586-023-06226-x
M3 - Article
C2 - 37587297
AN - SCOPUS:85168240026
SN - 0028-0836
VL - 620
SP - 525
EP - 532
JO - Nature
JF - Nature
IS - 7974
ER -