Quantum spin liquid in frustrated one-dimensional LiCuSbO 4

S. E. Dutton; M. Kumar; M. Mourigal; Z. G. Soos; J. J. Wen; C. L. Broholm; N. H. Andersen; Q. Huang; M. Zbiri; R. Toft-Petersen; R. J. Cava

doi:10.1103/PhysRevLett.108.187206

Quantum spin liquid in frustrated one-dimensional LiCuSbO ₄

S. E. Dutton
, M. Kumar
, M. Mourigal
, Z. G. Soos
, J. J. Wen
, C. L. Broholm
, N. H. Andersen
, Q. Huang
, M. Zbiri
, R. Toft-Petersen
, R. J. Cava

Research output: Contribution to journal › Article › peer-review

88 Scopus citations

Abstract

A quantum magnet, LiCuSbO ₄, with chains of edge-sharing spin-12 CuO ₆ octahedra is reported. While short-range order is observed for T<10K, no zero-field phase transition or spin freezing occurs down to 100mK. Specific heat indicates a distinct high-field phase near the 12T saturation field. Neutron scattering shows incommensurate spin correlations with q=(0.47±0.01)π/a and places an upper limit of 70μeV on any spin gap. Exact diagonalization of 16-spin easy-plane spin-12 chains with competing ferro- and antiferromagnetic interactions (J ₁=-75K, J ₂=34K) accounts for the T>2K data.

Original language	English (US)
Article number	187206
Journal	Physical review letters
Volume	108
Issue number	18
DOIs	https://doi.org/10.1103/PhysRevLett.108.187206
State	Published - May 3 2012

All Science Journal Classification (ASJC) codes

General Physics and Astronomy

Access to Document

10.1103/PhysRevLett.108.187206

Cite this

@article{e86633cd34ae4ba0a11d7cb0b2f37f4f,

title = "Quantum spin liquid in frustrated one-dimensional LiCuSbO 4 ",

abstract = "A quantum magnet, LiCuSbO 4, with chains of edge-sharing spin-12 CuO 6 octahedra is reported. While short-range order is observed for T<10K, no zero-field phase transition or spin freezing occurs down to 100mK. Specific heat indicates a distinct high-field phase near the 12T saturation field. Neutron scattering shows incommensurate spin correlations with q=(0.47±0.01)π/a and places an upper limit of 70μeV on any spin gap. Exact diagonalization of 16-spin easy-plane spin-12 chains with competing ferro- and antiferromagnetic interactions (J 1=-75K, J 2=34K) accounts for the T>2K data.",

author = "Dutton, \{S. E.\} and M. Kumar and M. Mourigal and Soos, \{Z. G.\} and Wen, \{J. J.\} and Broholm, \{C. L.\} and Andersen, \{N. H.\} and Q. Huang and M. Zbiri and R. Toft-Petersen and Cava, \{R. J.\}",

year = "2012",

month = may,

day = "3",

doi = "10.1103/PhysRevLett.108.187206",

language = "English (US)",

volume = "108",

journal = "Physical review letters",

issn = "0031-9007",

publisher = "American Physical Society",

number = "18",

}

TY - JOUR

T1 - Quantum spin liquid in frustrated one-dimensional LiCuSbO 4

AU - Dutton, S. E.

AU - Kumar, M.

AU - Mourigal, M.

AU - Soos, Z. G.

AU - Wen, J. J.

AU - Broholm, C. L.

AU - Andersen, N. H.

AU - Huang, Q.

AU - Zbiri, M.

AU - Toft-Petersen, R.

AU - Cava, R. J.

PY - 2012/5/3

Y1 - 2012/5/3

N2 - A quantum magnet, LiCuSbO 4, with chains of edge-sharing spin-12 CuO 6 octahedra is reported. While short-range order is observed for T<10K, no zero-field phase transition or spin freezing occurs down to 100mK. Specific heat indicates a distinct high-field phase near the 12T saturation field. Neutron scattering shows incommensurate spin correlations with q=(0.47±0.01)π/a and places an upper limit of 70μeV on any spin gap. Exact diagonalization of 16-spin easy-plane spin-12 chains with competing ferro- and antiferromagnetic interactions (J 1=-75K, J 2=34K) accounts for the T>2K data.

AB - A quantum magnet, LiCuSbO 4, with chains of edge-sharing spin-12 CuO 6 octahedra is reported. While short-range order is observed for T<10K, no zero-field phase transition or spin freezing occurs down to 100mK. Specific heat indicates a distinct high-field phase near the 12T saturation field. Neutron scattering shows incommensurate spin correlations with q=(0.47±0.01)π/a and places an upper limit of 70μeV on any spin gap. Exact diagonalization of 16-spin easy-plane spin-12 chains with competing ferro- and antiferromagnetic interactions (J 1=-75K, J 2=34K) accounts for the T>2K data.

UR - https://www.scopus.com/pages/publications/84860641783

UR - https://www.scopus.com/pages/publications/84860641783#tab=citedBy

U2 - 10.1103/PhysRevLett.108.187206

DO - 10.1103/PhysRevLett.108.187206

M3 - Article

C2 - 22681114

AN - SCOPUS:84860641783

SN - 0031-9007

VL - 108

JO - Physical review letters

JF - Physical review letters

IS - 18

M1 - 187206

ER -

Quantum spin liquid in frustrated one-dimensional LiCuSbO ₄

Abstract

All Science Journal Classification (ASJC) codes

Access to Document

Other files and links

Fingerprint

Cite this