Quantum spin dynamics of the honeycomb magnet K2Co2TeO6 in high magnetic fields

  • Patrick Pilch
  • , Laur Peedu
  • , Urmas Nagel
  • , Toomas Rõõm
  • , Changqing Zhu
  • , Yurii Skourski
  • , Xianghan Xu
  • , Robert J. Cava
  • , Zhe Wang

Research output: Contribution to journalArticlepeer-review

Abstract

We present terahertz spectroscopic measurements of quantum spin dynamics in the honeycomb magnet K2Co2TeO6 as a function of temperature, polarization and in an external magnetic field applied in the honeycomb plane. Magnetic excitations are resolved below the magnetic ordering temperature of TN = 12 K. In the applied magnetic field, we reveal characteristic field dependence not only for the magnetic excitations observed at zero field but also a rich set of modes emerging in finite fields. The observed magnetic excitations exhibit clear dependence on the terahertz polarization and characteristic features at field-induced phase transitions consistent with our high-field magnetization data. We cannot evidently resolve a continuumlike feature, even when the long-range magnetic order is presumably suppressed in the strong magnetic field, indicating that a Kitaev-type interaction, if existing, is subleading in this compound.

Original languageEnglish (US)
Article number014455
JournalPhysical Review B
Volume112
Issue number1
DOIs
StatePublished - Jul 31 2025

All Science Journal Classification (ASJC) codes

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

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