Quantum optimal control of multiple targets: Development of a monotonically convergent algorithm and application to intramolecular vibrational energy redistribution control

Yukiyoshi Ohtsuki; Kazuyuki Nakagami; Yuichi Fujimura; Wusheng Zhu; Herschel Rabitz

doi:10.1063/1.1368133

Quantum optimal control of multiple targets: Development of a monotonically convergent algorithm and application to intramolecular vibrational energy redistribution control

Yukiyoshi Ohtsuki, Kazuyuki Nakagami, Yuichi Fujimura, Wusheng Zhu, Herschel Rabitz

Research output: Contribution to journal › Article › peer-review

63 Scopus citations

Abstract

A new efficient algorithm was proposed for solving coupled quantum control equations allowing multiple target operators with desired expected values to specify an objective state. To design a field that transferred a molecule to an objective state an optimal control procedure was presented. Constraints on the time behavior of specified operators during the control period were taken into account. The algorithm represented in the quadruple-space notation reduced to double-space notation in the absence of time-dependant constraints.

Original language	English (US)
Pages (from-to)	8867-8876
Number of pages	10
Journal	Journal of Chemical Physics
Volume	114
Issue number	20
DOIs	https://doi.org/10.1063/1.1368133
State	Published - May 22 2001

All Science Journal Classification (ASJC) codes

General Physics and Astronomy
Physical and Theoretical Chemistry

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10.1063/1.1368133

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abstract = "A new efficient algorithm was proposed for solving coupled quantum control equations allowing multiple target operators with desired expected values to specify an objective state. To design a field that transferred a molecule to an objective state an optimal control procedure was presented. Constraints on the time behavior of specified operators during the control period were taken into account. The algorithm represented in the quadruple-space notation reduced to double-space notation in the absence of time-dependant constraints.",

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Quantum optimal control of multiple targets: Development of a monotonically convergent algorithm and application to intramolecular vibrational energy redistribution control. / Ohtsuki, Yukiyoshi; Nakagami, Kazuyuki; Fujimura, Yuichi et al.
In: Journal of Chemical Physics, Vol. 114, No. 20, 22.05.2001, p. 8867-8876.

Research output: Contribution to journal › Article › peer-review

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T1 - Quantum optimal control of multiple targets

T2 - Development of a monotonically convergent algorithm and application to intramolecular vibrational energy redistribution control

AU - Ohtsuki, Yukiyoshi

AU - Nakagami, Kazuyuki

AU - Fujimura, Yuichi

AU - Zhu, Wusheng

AU - Rabitz, Herschel

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Quantum optimal control of multiple targets: Development of a monotonically convergent algorithm and application to intramolecular vibrational energy redistribution control

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