TY - JOUR
T1 - Process systems engineering studies for the synthesis of catalytic biomass-to-fuels strategies
AU - Han, Jeehoon
AU - Murat Sen, S.
AU - Luterbacher, Jeremy S.
AU - Alonso, David Martin
AU - Dumesic, James A.
AU - Maravelias, Christos T.
N1 - Funding Information:
This work was funded by the DOE Great Lakes Bioenergy Research Center ( DOE BER Office of Science DE-FC02-07ER64494 ).
Publisher Copyright:
© 2015 Elsevier Ltd.
PY - 2014/11/5
Y1 - 2014/11/5
N2 - The goal of this paper is to show how chemical process synthesis and analysis studies can be coupled with experimental heterogeneous catalysis studies to identify promising research directions for the development of strategies for the production of renewable fuels. We study five catalytic biomass-to-fuels strategies that rely on production of platform chemicals, such as levulinic acid and fermentable sugars. We first integrate catalytic conversion subsystems with separation subsystems to generate complete conversion strategies, and we then develop the corresponding process simulation models based on experimental results. Our analyses suggest that catalytic biomass-to-fuel conversion strategies could become economically competitive alternatives to current biofuel production approaches as a result of iterative experimental and computational efforts.
AB - The goal of this paper is to show how chemical process synthesis and analysis studies can be coupled with experimental heterogeneous catalysis studies to identify promising research directions for the development of strategies for the production of renewable fuels. We study five catalytic biomass-to-fuels strategies that rely on production of platform chemicals, such as levulinic acid and fermentable sugars. We first integrate catalytic conversion subsystems with separation subsystems to generate complete conversion strategies, and we then develop the corresponding process simulation models based on experimental results. Our analyses suggest that catalytic biomass-to-fuel conversion strategies could become economically competitive alternatives to current biofuel production approaches as a result of iterative experimental and computational efforts.
KW - Heterogeneous catalysis
KW - Lignocellulosic biofuels
KW - Process synthesis
KW - Technoeconomic evaluation
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U2 - 10.1016/j.compchemeng.2015.04.007
DO - 10.1016/j.compchemeng.2015.04.007
M3 - Article
AN - SCOPUS:84947036098
SN - 0098-1354
VL - 81
SP - 57
EP - 69
JO - Computers and Chemical Engineering
JF - Computers and Chemical Engineering
ER -