Abstract
We reinvestigate the famous Mollow triplet and show that most of the well-known quantum characteristics of the Mollow triplet - including incoherent emission and a nonstandard dependence of the sidebands on detuning - can be recovered quantitatively using semiclassical dynamics with a classical light field. In fact, by not relying on the rotating wave approximation, a semiclassical model predicts some quantum effects beyond the quantum optical Bloch equation, including higher-order scattering and asymmetric sideband features. This Letter highlights the fact that, with strong intensities, many putatively quantum features of light-matter interactions arise from a simple balance of mean-field electrodynamics and elementary spontaneous emission, which requires minimal computational cost. Our results suggest that the application of semiclassical electrodynamics to problems with strong light-matter coupling in the fields of nanophotonics and superradiance are likely to yield a plethora of new information.
| Original language | English (US) |
|---|---|
| Pages (from-to) | 1331-1336 |
| Number of pages | 6 |
| Journal | Journal of Physical Chemistry Letters |
| Volume | 10 |
| Issue number | 6 |
| DOIs | |
| State | Published - Mar 21 2019 |
| Externally published | Yes |
All Science Journal Classification (ASJC) codes
- General Materials Science
- Physical and Theoretical Chemistry
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