Photoacoustic spectroscopy using quantum-cascade lasers

B. A. Paldus, T. G. Spence, R. N. Zare, J. Oomens, F. J.M. Harren, D. H. Parker, C. Gmachl, F. Cappasso, D. L. Sivco, J. N. Baillargeon, A. L. Hutchinson, A. Y. Cho

Research output: Contribution to journalArticlepeer-review

147 Scopus citations

Abstract

Photoacoustic spectra of ammonia and water vapor were recorded by use of a continuous-wave quantum-cascade distributed-feedback (QC-DFB) laser at 8.5 μmn with a 16-mW power output. The gases were flowed through a cell that was resonant at 1.6 kHz, and the QC-DFB source was temperature tuned over 35 nm for generation of spectra or was temperature stabilized on an absorption feature peak to permit real-time concentration measurements. A detection limit of 100 parts in 109 by volume ammonia at standard temperature and pressure was obtained for a 1-Hz bandwidth in a measurement time of 10 min.

Original languageEnglish (US)
Pages (from-to)178-180
Number of pages3
JournalOptics Letters
Volume24
Issue number3
DOIs
StatePublished - Feb 1 1999
Externally publishedYes

All Science Journal Classification (ASJC) codes

  • Atomic and Molecular Physics, and Optics

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