Ozone air quality and radiative forcing consequences of changes in ozone precursor emissions

J. Jason West, Arlene M. Fiore, Vaishali Naik, Larry W. Horowitz, M. Daniel Schwarzkopf, Denise Leonore Mauzerall

Research output: Contribution to journalArticlepeer-review

48 Scopus citations

Abstract

Changes in emissions of ozone (O3) precursors affect both air quality and climate. We first examine the sensitivity of surface O3 concentrations (O3srf) and net radiative forcing of climate (RFnet) to reductions in emissions of four precursors - nitrogen oxides (NOx), non-methane volatile organic compounds, carbon monoxide, and methane (CH4). We show that long-term CH4-induced changes in O3, known to be important for climate, are also relevant for air quality; for example, NOx reductions increase CH4, causing a long-term O3 increase that partially counteracts the direct O3 decrease. Second, we assess the radiative forcing resulting from actions to improve O3 air quality by calculating the ratio of ΔRFnet to changes in metrics of O3 srf. Decreases in CH4 emissions cause the greatest RFnet decrease per unit reduction in O3 srf, while NOx reductions increase RFnet. Of the available means to improve O3 air quality, therefore, CH4 abatement best reduces climate forcing.

Original languageEnglish (US)
Article numberL06806
JournalGeophysical Research Letters
Volume34
Issue number6
DOIs
StatePublished - Mar 28 2007

All Science Journal Classification (ASJC) codes

  • Geophysics
  • Earth and Planetary Sciences(all)

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