Abstract
The dynamical advantages for employing up to three independently shaped polarization fields are explored in the optimal control of quantum systems. The analysis compares multi-polarization optimal control with what may be achieved using linearly polarized (1-D) control. Simulations on model systems show how multi-polarization (2-D, 3-D) optimally shaped pulses can overcome symmetry forbidden transitions and improve control quality by better accessibility to the target state.
Original language | English (US) |
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Pages (from-to) | 469-475 |
Number of pages | 7 |
Journal | Chemical Physics Letters |
Volume | 400 |
Issue number | 4-6 |
DOIs | |
State | Published - Dec 21 2004 |
All Science Journal Classification (ASJC) codes
- General Physics and Astronomy
- Physical and Theoretical Chemistry