The dynamical advantages for employing up to three independently shaped polarization fields are explored in the optimal control of quantum systems. The analysis compares multi-polarization optimal control with what may be achieved using linearly polarized (1-D) control. Simulations on model systems show how multi-polarization (2-D, 3-D) optimally shaped pulses can overcome symmetry forbidden transitions and improve control quality by better accessibility to the target state.
|Original language||English (US)|
|Number of pages||7|
|Journal||Chemical Physics Letters|
|State||Published - Dec 21 2004|
All Science Journal Classification (ASJC) codes
- Physics and Astronomy(all)
- Physical and Theoretical Chemistry