Optimal Hamiltonian identification: The synthesis of quantum optimal control and quantum inversion

J. M. Geremia, Herschel Albert Rabitz

Research output: Contribution to journalArticlepeer-review

24 Scopus citations

Abstract

The concept of OI was introduced and demonstrated using the particular example of extracting transition dipole moment matrix elements from population transfer experimental data. It was confirmed that OI for extracting Hamiltonian information combines the strongest features of both modern laser control experiments and nonlinear inversion techniques to make use of global searching, high experimental repetition rates and ultrafast pulse shaping technology to actively probe the quantum Hamiltonian and reveal the optimal data set for performing an identification.

Original languageEnglish (US)
Pages (from-to)5369-5382
Number of pages14
JournalJournal of Chemical Physics
Volume118
Issue number12
DOIs
StatePublished - Mar 22 2003

All Science Journal Classification (ASJC) codes

  • Physics and Astronomy(all)
  • Physical and Theoretical Chemistry

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