Abstract
We show that the strongly spin-orbit coupled materials Bi2Te3 and Sb2Te3 and their derivatives belong to the Z2 topological-insulator class. Using a combination of first-principles theoretical calculations and photoemission spectroscopy, we directly show that Bi2Te3 is a large spin-orbit-induced indirect bulk band gap (δ∼150meV) semiconductor whose surface is characterized by a single topological spin-Dirac cone. The electronic structure of self-doped Sb2Te3 exhibits similar Z2 topological properties. We demonstrate that the dynamics of spin-Dirac fermions can be controlled through systematic Mn doping, making these materials classes potentially suitable for topological device applications.
Original language | English (US) |
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Article number | 146401 |
Journal | Physical review letters |
Volume | 103 |
Issue number | 14 |
DOIs | |
State | Published - Sep 28 2009 |
All Science Journal Classification (ASJC) codes
- General Physics and Astronomy