Observable-preserving control of quantum dynamics over a family of related systems

Adam Rothman, Tak San Ho, Herschel Albert Rabitz

Research output: Contribution to journalArticle

65 Scopus citations

Abstract

Quantum control aims at the manipulation of atomic- and molecular-scale dynamics phenomena. An important objective in this regard is the understanding of dynamical control within a family of related quantum systems. To explore this issue, diffeomorphic changes in the system Hamiltonian H(s,t) are introduced by scanning over a homotopy parameter s and then monitoring the control field response needed to maintain the value of a specified target observable. This operation is implemented through a procedure referred to as diffeomorphic modulation under observable-response-preserving homotopy (D-MORPH). The governing D-MORPH differential equation determining the control laser field E(s,t) is shown to explicitly allow for innumerable solutions, with each characterized by the choice of an arbitrary function f(s,t) of and time t. The presence of f(s,t) in the D-MORPH differential equation makes clear the origin of multiple control fields that produce the same observable objective. A stable algorithm is presented for practical execution of D-MORPH with the only criterion that the Hamiltonian H(s,t) permit reaching the objective over the full domain of s being sampled. Both analytic and numerical examples are presented to illustrate the D-MORPH concept.

Original languageEnglish (US)
Article number023416
JournalPhysical Review A - Atomic, Molecular, and Optical Physics
Volume72
Issue number2
DOIs
StatePublished - Aug 1 2005

All Science Journal Classification (ASJC) codes

  • Atomic and Molecular Physics, and Optics

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