Nonlinear optical properties of the inorganic metal cluster MO2Ag4S8(PPh3)4

Tiejun Xia, Arthur Dogariu, K. Mansour, David J. Hagan, Ali A. Said, Eric W. Van Stryland, Shu Shi

Research output: Chapter in Book/Report/Conference proceedingConference contribution

9 Scopus citations

Abstract

We describe a series of experiments on solutions of the inorganic metal cluster molecules Mo 2Ag 4S 8(PPh 3) 4 and compare them with data on a suspension of carbon particles in liquid (ink). The optical limiting behavior is measured using both single picosecond 532 nm pulses and nanosecond long trains of these picosecond pulses. Both materials show reduced transmittance for increasing fluence (energy per unit area). We also perform picosecond time-resolved pump-probe measurements. We find that the observed pump-probe data is nearly identical for the metal cluster solution and the carbon particle suspension (CBS), and we conclude that the nonlinear mechanisms are the same for the two materials. Our previous studies have shown that the nonlinear losses are due to scattering and absorption by microplasmas formed after thermionic emission from heated particles of carbon or inorganic clusters.

Original languageEnglish (US)
Title of host publicationProceedings of SPIE - The International Society for Optical Engineering
EditorsChristopher M. Lawson
Pages142-148
Number of pages7
StatePublished - Dec 1 1996
Externally publishedYes
EventNonlinear Optical Liquids - Denver, CO, USA
Duration: Aug 5 1996Aug 6 1996

Publication series

NameProceedings of SPIE - The International Society for Optical Engineering
Volume2853
ISSN (Print)0277-786X

Other

OtherNonlinear Optical Liquids
CityDenver, CO, USA
Period8/5/968/6/96

All Science Journal Classification (ASJC) codes

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics
  • Computer Science Applications
  • Applied Mathematics
  • Electrical and Electronic Engineering

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