NbIr2B2 and TaIr2B2 – New Low Symmetry Noncentrosymmetric Superconductors with Strong Spin–Orbit Coupling

Karolina Górnicka, Xin Gui, Bartlomiej Wiendlocha, Loi T. Nguyen, Weiwei Xie, Robert J. Cava, Tomasz Klimczuk

Research output: Contribution to journalArticlepeer-review

1 Scopus citations

Abstract

Superconductivity was first observed more than a century ago, but the search for new superconducting materials remains a challenge. The Cooper pairs in superconductors are ideal embodiments of quantum entanglement. Thus, novel superconductors can be critical for both learning about electronic systems in condensed matter and for possible application in future quantum technologies. Here two previously unreported materials, NbIr2B2 and TaIr2B2, are presented with superconducting transitions at 7.2 and 5.2 K, respectively. They display a unique noncentrosymmetric crystal structure, and for both compounds the magnetic field that destroys the superconductivity at 0 K exceeds one of the fundamental characteristics of conventional superconductors (the “Pauli limit”), suggesting that the superconductivity may be unconventional. Supporting this experimentally based deduction, first-principle calculations show a spin-split Fermi surface due to the presence of strong spin–orbit coupling. These materials may thus provide an excellent platform for the study of unconventional superconductivity in intermetallic compounds.

Original languageEnglish (US)
Article number2007960
JournalAdvanced Functional Materials
Volume31
Issue number3
DOIs
StatePublished - Jan 18 2021

All Science Journal Classification (ASJC) codes

  • Chemistry(all)
  • Materials Science(all)
  • Condensed Matter Physics

Keywords

  • crystal structure
  • noncentrosymmetric superconductors
  • spin–orbit coupling

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