Highly efficient perovskite solar cells with crosslinked PCBM interlayers

W. Qiu; J. P. Bastos; S. Dasgupta; T. Merckx; I. Cardinaletti; M. V.C. Jenart; C. B. Nielsen; R. Gehlhaar; J. Poortmans; P. Heremans; I. McCulloch; D. Cheyns

doi:10.1039/c6ta08799j

Highly efficient perovskite solar cells with crosslinked PCBM interlayers

W. Qiu, J. P. Bastos, S. Dasgupta, T. Merckx, I. Cardinaletti, M. V.C. Jenart, C. B. Nielsen, R. Gehlhaar, J. Poortmans, P. Heremans, I. McCulloch, D. Cheyns

Research output: Contribution to journal › Article › peer-review

54 Scopus citations

Abstract

Commercially available phenyl-C₆₁-butyric acid methyl ester (PCBM) is crosslinked with 1,6-diazidohexane (DAZH), resulting in films resistant to common solvents used in perovskite solar cell processing. By using crosslinked PCBM as an interlayer and (HC(NH₂)₂)_0.66(CH₃NH₃)_0.34PbI_2.85Br_0.15 as the active layer, we achieve small area devices and modules with a maximum steady-state power conversion efficiency of 18.1% and 14.9%, respectively.

Original language	English (US)
Pages (from-to)	2466-2472
Number of pages	7
Journal	Journal of Materials Chemistry A
Volume	5
Issue number	6
DOIs	https://doi.org/10.1039/c6ta08799j
State	Published - 2017
Externally published	Yes

All Science Journal Classification (ASJC) codes

General Chemistry
Renewable Energy, Sustainability and the Environment
General Materials Science

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10.1039/c6ta08799j

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title = "Highly efficient perovskite solar cells with crosslinked PCBM interlayers",

abstract = "Commercially available phenyl-C61-butyric acid methyl ester (PCBM) is crosslinked with 1,6-diazidohexane (DAZH), resulting in films resistant to common solvents used in perovskite solar cell processing. By using crosslinked PCBM as an interlayer and (HC(NH2)2)0.66(CH3NH3)0.34PbI2.85Br0.15 as the active layer, we achieve small area devices and modules with a maximum steady-state power conversion efficiency of 18.1% and 14.9%, respectively.",

author = "W. Qiu and Bastos, {J. P.} and S. Dasgupta and T. Merckx and I. Cardinaletti and Jenart, {M. V.C.} and Nielsen, {C. B.} and R. Gehlhaar and J. Poortmans and P. Heremans and I. McCulloch and D. Cheyns",

note = "Publisher Copyright: {\textcopyright} The Royal Society of Chemistry.",

year = "2017",

doi = "10.1039/c6ta08799j",

language = "English (US)",

volume = "5",

pages = "2466--2472",

journal = "Journal of Materials Chemistry A",

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TY - JOUR

T1 - Highly efficient perovskite solar cells with crosslinked PCBM interlayers

AU - Qiu, W.

AU - Bastos, J. P.

AU - Dasgupta, S.

AU - Merckx, T.

AU - Cardinaletti, I.

AU - Jenart, M. V.C.

AU - Nielsen, C. B.

AU - Gehlhaar, R.

AU - Poortmans, J.

AU - Heremans, P.

AU - McCulloch, I.

AU - Cheyns, D.

PY - 2017

Y1 - 2017

N2 - Commercially available phenyl-C61-butyric acid methyl ester (PCBM) is crosslinked with 1,6-diazidohexane (DAZH), resulting in films resistant to common solvents used in perovskite solar cell processing. By using crosslinked PCBM as an interlayer and (HC(NH2)2)0.66(CH3NH3)0.34PbI2.85Br0.15 as the active layer, we achieve small area devices and modules with a maximum steady-state power conversion efficiency of 18.1% and 14.9%, respectively.

AB - Commercially available phenyl-C61-butyric acid methyl ester (PCBM) is crosslinked with 1,6-diazidohexane (DAZH), resulting in films resistant to common solvents used in perovskite solar cell processing. By using crosslinked PCBM as an interlayer and (HC(NH2)2)0.66(CH3NH3)0.34PbI2.85Br0.15 as the active layer, we achieve small area devices and modules with a maximum steady-state power conversion efficiency of 18.1% and 14.9%, respectively.

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DO - 10.1039/c6ta08799j

M3 - Article

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JO - Journal of Materials Chemistry A

JF - Journal of Materials Chemistry A

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ER -

Highly efficient perovskite solar cells with crosslinked PCBM interlayers

Abstract

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