High-performance perovskite single-junction and textured perovskite/silicon tandem solar cells via slot-die-coating

Anand S. Subbiah; Furkan H. Isikgor; Calvyn T. Howells; Michele De Bastiani; Jiang Liu; Erkan Aydin; Francesco Furlan; Thomas G. Allen; Fuzong Xu; Shynggys Zhumagali; Sjoerd Hoogland; Edward H. Sargent; Iain McCulloch; Stefaan De Wolf

doi:10.1021/acsenergylett.0c01297

High-performance perovskite single-junction and textured perovskite/silicon tandem solar cells via slot-die-coating

Anand S. Subbiah
, Furkan H. Isikgor
, Calvyn T. Howells
, Michele De Bastiani
, Jiang Liu
, Erkan Aydin
, Francesco Furlan
, Thomas G. Allen
, Fuzong Xu
, Shynggys Zhumagali
, Sjoerd Hoogland
, Edward H. Sargent
, Iain McCulloch
, Stefaan De Wolf

Research output: Contribution to journal › Article › peer-review

182 Scopus citations

Abstract

In this work, we report perovskite solar cells in the planar p-i-n configuration based on single-step, anti-solvent-free, low-temperature (70 °C) slot-die-coated methylammonium lead tri-iodide (MAPbI3). The devices are fabricated on hydrophobic poly(triarylamine) (PTAA) surfaces, using key strategies such as solvent engineering, enhanced ink-substrate dynamics, and surface passivation, enabling a power conversion efficiency (PCE) of 21.8%. We also adapted the technique to achieve the first slot-die-coated perovskite/silicon monolithic 2-terminal tandems, achieving a PCE of 23.8% utilizing a textured silicon bottom cell.

Original language	English (US)
Pages (from-to)	3034-3040
Number of pages	7
Journal	ACS Energy Letters
Volume	5
Issue number	9
DOIs	https://doi.org/10.1021/acsenergylett.0c01297
State	Published - Sep 11 2020
Externally published	Yes

All Science Journal Classification (ASJC) codes

Chemistry (miscellaneous)
Renewable Energy, Sustainability and the Environment
Fuel Technology
Energy Engineering and Power Technology
Materials Chemistry

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10.1021/acsenergylett.0c01297

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Subbiah, A. S., Isikgor, F. H., Howells, C. T., De Bastiani, M., Liu, J., Aydin, E., Furlan, F., Allen, T. G., Xu, F., Zhumagali, S., Hoogland, S., Sargent, E. H., McCulloch, I., & De Wolf, S. (2020). High-performance perovskite single-junction and textured perovskite/silicon tandem solar cells via slot-die-coating. ACS Energy Letters, 5(9), 3034-3040. https://doi.org/10.1021/acsenergylett.0c01297

@article{58fcf755ab774ddcacb90336fc45ec21,

title = "High-performance perovskite single-junction and textured perovskite/silicon tandem solar cells via slot-die-coating",

abstract = "In this work, we report perovskite solar cells in the planar p-i-n configuration based on single-step, anti-solvent-free, low-temperature (70 °C) slot-die-coated methylammonium lead tri-iodide (MAPbI3). The devices are fabricated on hydrophobic poly(triarylamine) (PTAA) surfaces, using key strategies such as solvent engineering, enhanced ink-substrate dynamics, and surface passivation, enabling a power conversion efficiency (PCE) of 21.8\%. We also adapted the technique to achieve the first slot-die-coated perovskite/silicon monolithic 2-terminal tandems, achieving a PCE of 23.8\% utilizing a textured silicon bottom cell.",

author = "Subbiah, \{Anand S.\} and Isikgor, \{Furkan H.\} and Howells, \{Calvyn T.\} and \{De Bastiani\}, Michele and Jiang Liu and Erkan Aydin and Francesco Furlan and Allen, \{Thomas G.\} and Fuzong Xu and Shynggys Zhumagali and Sjoerd Hoogland and Sargent, \{Edward H.\} and Iain McCulloch and \{De Wolf\}, Stefaan",

note = "Publisher Copyright: Copyright {\textcopyright} 2020 American Chemical Society.",

year = "2020",

month = sep,

day = "11",

doi = "10.1021/acsenergylett.0c01297",

language = "English (US)",

volume = "5",

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Subbiah, AS, Isikgor, FH, Howells, CT, De Bastiani, M, Liu, J, Aydin, E, Furlan, F, Allen, TG, Xu, F, Zhumagali, S, Hoogland, S, Sargent, EH, McCulloch, I & De Wolf, S 2020, 'High-performance perovskite single-junction and textured perovskite/silicon tandem solar cells via slot-die-coating', ACS Energy Letters, vol. 5, no. 9, pp. 3034-3040. https://doi.org/10.1021/acsenergylett.0c01297

TY - JOUR

T1 - High-performance perovskite single-junction and textured perovskite/silicon tandem solar cells via slot-die-coating

AU - Subbiah, Anand S.

AU - Isikgor, Furkan H.

AU - Howells, Calvyn T.

AU - De Bastiani, Michele

AU - Liu, Jiang

AU - Aydin, Erkan

AU - Furlan, Francesco

AU - Allen, Thomas G.

AU - Xu, Fuzong

AU - Zhumagali, Shynggys

AU - Hoogland, Sjoerd

AU - Sargent, Edward H.

AU - McCulloch, Iain

AU - De Wolf, Stefaan

PY - 2020/9/11

Y1 - 2020/9/11

N2 - In this work, we report perovskite solar cells in the planar p-i-n configuration based on single-step, anti-solvent-free, low-temperature (70 °C) slot-die-coated methylammonium lead tri-iodide (MAPbI3). The devices are fabricated on hydrophobic poly(triarylamine) (PTAA) surfaces, using key strategies such as solvent engineering, enhanced ink-substrate dynamics, and surface passivation, enabling a power conversion efficiency (PCE) of 21.8%. We also adapted the technique to achieve the first slot-die-coated perovskite/silicon monolithic 2-terminal tandems, achieving a PCE of 23.8% utilizing a textured silicon bottom cell.

AB - In this work, we report perovskite solar cells in the planar p-i-n configuration based on single-step, anti-solvent-free, low-temperature (70 °C) slot-die-coated methylammonium lead tri-iodide (MAPbI3). The devices are fabricated on hydrophobic poly(triarylamine) (PTAA) surfaces, using key strategies such as solvent engineering, enhanced ink-substrate dynamics, and surface passivation, enabling a power conversion efficiency (PCE) of 21.8%. We also adapted the technique to achieve the first slot-die-coated perovskite/silicon monolithic 2-terminal tandems, achieving a PCE of 23.8% utilizing a textured silicon bottom cell.

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SN - 2380-8195

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SP - 3034

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JO - ACS Energy Letters

JF - ACS Energy Letters

IS - 9

ER -

High-performance perovskite single-junction and textured perovskite/silicon tandem solar cells via slot-die-coating

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