TY - JOUR
T1 - High-entropy nanoparticles
T2 - Synthesis-structureproperty relationships and data-driven discovery
AU - Yao, Yonggang
AU - Dong, Qi
AU - Brozena, Alexandra
AU - Luo, Jian
AU - Miao, Jianwei
AU - Chi, Miaofang
AU - Wang, Chao
AU - Kevrekidis, Yannis
AU - Ren, Zhiyong Jason
AU - Greeley, Jeffrey
AU - Wang, Guofeng
AU - Anapolsky, Abraham
AU - Hu, Liangbing
N1 - Publisher Copyright:
© 2022 American Association for the Advancement of Science. All rights reserved.
PY - 2022/4/8
Y1 - 2022/4/8
N2 - High-entropy nanoparticles have become a rapidly growing area of research in recent years. Because of their multielemental compositions and unique high-entropy mixing states (i.e., solid-solution) that can lead to tunable activity and enhanced stability, these nanoparticles have received notable attention for catalyst design and exploration. However, this strong potential is also accompanied by grand challenges originating from their vast compositional space and complex atomic structure, which hinder comprehensive exploration and fundamental understanding. Through a multidisciplinary view of synthesis, characterization, catalytic applications, high-throughput screening, and data-driven materials discovery, this review is dedicated to discussing the important progress of high-entropy nanoparticles and unveiling the critical needs for their future development for catalysis, energy, and sustainability applications.
AB - High-entropy nanoparticles have become a rapidly growing area of research in recent years. Because of their multielemental compositions and unique high-entropy mixing states (i.e., solid-solution) that can lead to tunable activity and enhanced stability, these nanoparticles have received notable attention for catalyst design and exploration. However, this strong potential is also accompanied by grand challenges originating from their vast compositional space and complex atomic structure, which hinder comprehensive exploration and fundamental understanding. Through a multidisciplinary view of synthesis, characterization, catalytic applications, high-throughput screening, and data-driven materials discovery, this review is dedicated to discussing the important progress of high-entropy nanoparticles and unveiling the critical needs for their future development for catalysis, energy, and sustainability applications.
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U2 - 10.1126/science.abn3103
DO - 10.1126/science.abn3103
M3 - Review article
C2 - 35389801
AN - SCOPUS:85127892567
SN - 0036-8075
VL - 376
JO - Science
JF - Science
IS - 6589
M1 - abn3103
ER -