Abstract
A general set of quantitative model assessment and analysis tools, termed high-dimensional model representations (HDMR), have been introduced recently for high dimensional input-output systems. HDMR are a particular family of representations where each term in the representation reflects the independent and cooperative contributions of the inputs upon the output. When data are randomly sampled, a RS(random sampling)-HDMR can be constructed, which is an efficient tool to provide a fully global statistical analysis of a model. The individual RS-HDMR component functions have a direct statistical correlation interpretation. This relation permits the model output variance σ2 to be decomposed into its input contributions σ2 = Σiσ2i + Σi<j σ2ij +. due to the independent variable action σ2i, the pair correlation action σ2ij, etc. The information gained from this decomposition can be valuable for attaining a physical understanding of the origins of output uncertainty as well as suggesting additional laboratory/field studies or model refinements to best improve the quality of the model. To reduce sampling effort, the RS-HDMR component functions are approximately represented by orthonormal polynomials. Only one randomly sampled set of input-output data is needed to determine all σi, σij, etc. and a few hundred samples may give reliable results. This paper presents its methodology and applications on an atmospheric photochemistry model and a trace metal bioremediation model.
| Original language | English (US) |
|---|---|
| Pages (from-to) | 4445-4460 |
| Number of pages | 16 |
| Journal | Chemical Engineering Science |
| Volume | 57 |
| Issue number | 21 |
| DOIs | |
| State | Published - Nov 4 2002 |
All Science Journal Classification (ASJC) codes
- General Chemistry
- General Chemical Engineering
- Industrial and Manufacturing Engineering
Keywords
- Global uncertainty analysis
- High dimensional model representation
- Monte Carlo method
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