Electron spin coherence of phosphorus donors in silicon: Effect of environmental nuclei

Eisuke Abe; Alexei M. Tyryshkin; Shinichi Tojo; John J.L. Morton; Wayne M. Witzel; Akira Fujimoto; Joel W. Ager; Eugene E. Haller; Junichi Isoya; Stephen A. Lyon; Mike L.W. Thewalt; Kohei M. Itoh

doi:10.1103/PhysRevB.82.121201

Electron spin coherence of phosphorus donors in silicon: Effect of environmental nuclei

Eisuke Abe, Alexei M. Tyryshkin, Shinichi Tojo, John J.L. Morton, Wayne M. Witzel, Akira Fujimoto, Joel W. Ager, Eugene E. Haller, Junichi Isoya, Stephen A. Lyon, Mike L.W. Thewalt, Kohei M. Itoh

Research output: Contribution to journal › Article › peer-review

76 Scopus citations

Abstract

We report electron paramagnetic resonance (EPR) experiments of phosphorus donors in isotopically controlled silicon single crystals. By varying the concentration of the ²⁹Si isotope, f, from 0.075% to 99.2%, we systematically study the effect of the environmental nuclear spins on the donor-electron spin. We find excellent agreement between experiment and theory for decoherence times due to nuclear-induced spectral diffusion, clarifying that the nuclear-induced decoherence is dominant in the range of f studied. We also observe that the EPR linewidth shows a transition from the square-root dependence to the linear dependence on f, in agreement with theoretical predictions.

Original language	English (US)
Article number	121201
Journal	Physical Review B - Condensed Matter and Materials Physics
Volume	82
Issue number	12
DOIs	https://doi.org/10.1103/PhysRevB.82.121201
State	Published - Sep 2 2010

All Science Journal Classification (ASJC) codes

Electronic, Optical and Magnetic Materials
Condensed Matter Physics

Access to Document

10.1103/PhysRevB.82.121201

Cite this

Abe, E., Tyryshkin, A. M., Tojo, S., Morton, J. J. L., Witzel, W. M., Fujimoto, A., Ager, J. W., Haller, E. E., Isoya, J., Lyon, S. A., Thewalt, M. L. W., & Itoh, K. M. (2010). Electron spin coherence of phosphorus donors in silicon: Effect of environmental nuclei. Physical Review B - Condensed Matter and Materials Physics, 82(12), Article 121201. https://doi.org/10.1103/PhysRevB.82.121201

@article{66f32dd0c0f1457dbf753c2277465016,

title = "Electron spin coherence of phosphorus donors in silicon: Effect of environmental nuclei",

abstract = "We report electron paramagnetic resonance (EPR) experiments of phosphorus donors in isotopically controlled silicon single crystals. By varying the concentration of the 29Si isotope, f, from 0.075% to 99.2%, we systematically study the effect of the environmental nuclear spins on the donor-electron spin. We find excellent agreement between experiment and theory for decoherence times due to nuclear-induced spectral diffusion, clarifying that the nuclear-induced decoherence is dominant in the range of f studied. We also observe that the EPR linewidth shows a transition from the square-root dependence to the linear dependence on f, in agreement with theoretical predictions.",

author = "Eisuke Abe and Tyryshkin, {Alexei M.} and Shinichi Tojo and Morton, {John J.L.} and Witzel, {Wayne M.} and Akira Fujimoto and Ager, {Joel W.} and Haller, {Eugene E.} and Junichi Isoya and Lyon, {Stephen A.} and Thewalt, {Mike L.W.} and Itoh, {Kohei M.}",

year = "2010",

month = sep,

day = "2",

doi = "10.1103/PhysRevB.82.121201",

language = "English (US)",

volume = "82",

journal = "Physical Review B - Condensed Matter and Materials Physics",

issn = "1098-0121",

publisher = "American Physical Society",

number = "12",

}

TY - JOUR

T1 - Electron spin coherence of phosphorus donors in silicon

T2 - Effect of environmental nuclei

AU - Abe, Eisuke

AU - Tyryshkin, Alexei M.

AU - Tojo, Shinichi

AU - Morton, John J.L.

AU - Witzel, Wayne M.

AU - Fujimoto, Akira

AU - Ager, Joel W.

AU - Haller, Eugene E.

AU - Isoya, Junichi

AU - Lyon, Stephen A.

AU - Thewalt, Mike L.W.

AU - Itoh, Kohei M.

PY - 2010/9/2

Y1 - 2010/9/2

N2 - We report electron paramagnetic resonance (EPR) experiments of phosphorus donors in isotopically controlled silicon single crystals. By varying the concentration of the 29Si isotope, f, from 0.075% to 99.2%, we systematically study the effect of the environmental nuclear spins on the donor-electron spin. We find excellent agreement between experiment and theory for decoherence times due to nuclear-induced spectral diffusion, clarifying that the nuclear-induced decoherence is dominant in the range of f studied. We also observe that the EPR linewidth shows a transition from the square-root dependence to the linear dependence on f, in agreement with theoretical predictions.

AB - We report electron paramagnetic resonance (EPR) experiments of phosphorus donors in isotopically controlled silicon single crystals. By varying the concentration of the 29Si isotope, f, from 0.075% to 99.2%, we systematically study the effect of the environmental nuclear spins on the donor-electron spin. We find excellent agreement between experiment and theory for decoherence times due to nuclear-induced spectral diffusion, clarifying that the nuclear-induced decoherence is dominant in the range of f studied. We also observe that the EPR linewidth shows a transition from the square-root dependence to the linear dependence on f, in agreement with theoretical predictions.

UR - http://www.scopus.com/inward/record.url?scp=77957710211&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=77957710211&partnerID=8YFLogxK

U2 - 10.1103/PhysRevB.82.121201

DO - 10.1103/PhysRevB.82.121201

M3 - Article

AN - SCOPUS:77957710211

SN - 1098-0121

VL - 82

JO - Physical Review B - Condensed Matter and Materials Physics

JF - Physical Review B - Condensed Matter and Materials Physics

IS - 12

M1 - 121201

ER -

Electron spin coherence of phosphorus donors in silicon: Effect of environmental nuclei

Abstract

All Science Journal Classification (ASJC) codes

Access to Document

Other files and links

Fingerprint

Cite this