Effects of boundaries on pattern formation: Catalytic oxidation of CO on platinum

M. D. Graham; Ioannis G. Kevrekidis; K. Asakura; J. Lauterbach; K. Krischer; H. H. Rotermund; G. Ertl

doi:10.1126/science.264.5155.80

Effects of boundaries on pattern formation: Catalytic oxidation of CO on platinum

M. D. Graham, Ioannis G. Kevrekidis, K. Asakura, J. Lauterbach, K. Krischer, H. H. Rotermund, G. Ertl

Chemical & Biological Engineering

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133 Scopus citations

Abstract

The effect of boundaries on pattern formation was studied for the catalytic oxidation of carbon monoxide on platinum surfaces. Photolithography was used to create microscopic reacting domains on polycrystalline foils and single-crystal platinum (110) surfaces with inert titanium overlayers. Certain domain geometries give rise to patterns that have not been observed on the untreated catalyst and bring to light surface mechanisms that have no analog in homogeneous reaction-diffusion systems.

Original language	English (US)
Pages (from-to)	80-82
Number of pages	3
Journal	Science
Volume	264
Issue number	5155
DOIs	https://doi.org/10.1126/science.264.5155.80
State	Published - Apr 1 1994

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abstract = "The effect of boundaries on pattern formation was studied for the catalytic oxidation of carbon monoxide on platinum surfaces. Photolithography was used to create microscopic reacting domains on polycrystalline foils and single-crystal platinum (110) surfaces with inert titanium overlayers. Certain domain geometries give rise to patterns that have not been observed on the untreated catalyst and bring to light surface mechanisms that have no analog in homogeneous reaction-diffusion systems.",

author = "Graham, {M. D.} and Kevrekidis, {Ioannis G.} and K. Asakura and J. Lauterbach and K. Krischer and Rotermund, {H. H.} and G. Ertl",

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AU - Asakura, K.

AU - Lauterbach, J.

AU - Krischer, K.

AU - Rotermund, H. H.

AU - Ertl, G.

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AB - The effect of boundaries on pattern formation was studied for the catalytic oxidation of carbon monoxide on platinum surfaces. Photolithography was used to create microscopic reacting domains on polycrystalline foils and single-crystal platinum (110) surfaces with inert titanium overlayers. Certain domain geometries give rise to patterns that have not been observed on the untreated catalyst and bring to light surface mechanisms that have no analog in homogeneous reaction-diffusion systems.

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Effects of boundaries on pattern formation: Catalytic oxidation of CO on platinum

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