TY - JOUR
T1 - Dynamics of pattern coarsening in a two-dimensional smectic system
AU - Harrison, Christopher
AU - Cheng, Zhengdong
AU - Sethuraman, Srinivasan
AU - Huse, David A.
AU - Chaikin, Paul M.
AU - Vega, Daniel A.
AU - Sebastian, John M.
AU - Register, Richard A.
AU - Adamson, Douglas H.
PY - 2002/7/29
Y1 - 2002/7/29
N2 - We have followed the coarsening dynamics of a single layer of cylindrical block copolymer microdomains in a thin film. This system has the symmetry of a two-dimensional smectic. The orientational correlation length of the microdomains was measured by scanning electron microscopy and found to grow with the average spacing between [formula presented] disclinations, following a power law [formula presented] By tracking disclinations during annealing with time-lapse atomic force microscopy, we observe dominant mechanisms of disclination annihilation involving tripoles and quadrupoles (three and four disclinations, respectively). We describe how annihilation events involving multiple disclinations result in similarly reduced kinetic exponents as observed here. These results map onto a wide variety of physical systems that exhibit similarly striped patterns.
AB - We have followed the coarsening dynamics of a single layer of cylindrical block copolymer microdomains in a thin film. This system has the symmetry of a two-dimensional smectic. The orientational correlation length of the microdomains was measured by scanning electron microscopy and found to grow with the average spacing between [formula presented] disclinations, following a power law [formula presented] By tracking disclinations during annealing with time-lapse atomic force microscopy, we observe dominant mechanisms of disclination annihilation involving tripoles and quadrupoles (three and four disclinations, respectively). We describe how annihilation events involving multiple disclinations result in similarly reduced kinetic exponents as observed here. These results map onto a wide variety of physical systems that exhibit similarly striped patterns.
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U2 - 10.1103/PhysRevE.66.011706
DO - 10.1103/PhysRevE.66.011706
M3 - Article
C2 - 12241374
AN - SCOPUS:33749829783
SN - 1063-651X
VL - 66
JO - Physical Review E - Statistical Physics, Plasmas, Fluids, and Related Interdisciplinary Topics
JF - Physical Review E - Statistical Physics, Plasmas, Fluids, and Related Interdisciplinary Topics
IS - 1
ER -