Coulomb correlations, spectral line shapes, and size distributions of CdSe nanocrystals

Gregory D. Scholes; Margaret A. Hines; Anne Colonna; Mayrose Salvador

doi:10.1007/978-3-642-59319-2_115

Coulomb correlations, spectral line shapes, and size distributions of CdSe nanocrystals

Gregory D. Scholes, Margaret A. Hines, Anne Colonna, Mayrose Salvador

Research output: Contribution to journal › Article › peer-review

Abstract

We report 2-pulse and 3-pulse photon echo studies of CdSe nanocrystals at 293 K and 4.5 K. The data and simulations, which include the effects of many-particle correlations for the 2PE, show that the 3PE signal provides a precise measurement of the inhomogeneity in the exciton transition energy due to the size distribution of the quantum dots. The dephasing processes revealed by the 2PE are found to occur on at least two important time scales.

Original language	English (US)
Pages (from-to)	371-373
Number of pages	3
Journal	Springer Series in Chemical Physics
Volume	71
DOIs	https://doi.org/10.1007/978-3-642-59319-2_115
State	Published - 2003
Externally published	Yes

All Science Journal Classification (ASJC) codes

Physical and Theoretical Chemistry

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10.1007/978-3-642-59319-2_115

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title = "Coulomb correlations, spectral line shapes, and size distributions of CdSe nanocrystals",

abstract = "We report 2-pulse and 3-pulse photon echo studies of CdSe nanocrystals at 293 K and 4.5 K. The data and simulations, which include the effects of many-particle correlations for the 2PE, show that the 3PE signal provides a precise measurement of the inhomogeneity in the exciton transition energy due to the size distribution of the quantum dots. The dephasing processes revealed by the 2PE are found to occur on at least two important time scales.",

author = "Scholes, {Gregory D.} and Hines, {Margaret A.} and Anne Colonna and Mayrose Salvador",

year = "2003",

doi = "10.1007/978-3-642-59319-2_115",

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pages = "371--373",

journal = "Springer Series in Chemical Physics",

issn = "0172-6218",

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T1 - Coulomb correlations, spectral line shapes, and size distributions of CdSe nanocrystals

AU - Scholes, Gregory D.

AU - Hines, Margaret A.

AU - Colonna, Anne

AU - Salvador, Mayrose

PY - 2003

Y1 - 2003

N2 - We report 2-pulse and 3-pulse photon echo studies of CdSe nanocrystals at 293 K and 4.5 K. The data and simulations, which include the effects of many-particle correlations for the 2PE, show that the 3PE signal provides a precise measurement of the inhomogeneity in the exciton transition energy due to the size distribution of the quantum dots. The dephasing processes revealed by the 2PE are found to occur on at least two important time scales.

AB - We report 2-pulse and 3-pulse photon echo studies of CdSe nanocrystals at 293 K and 4.5 K. The data and simulations, which include the effects of many-particle correlations for the 2PE, show that the 3PE signal provides a precise measurement of the inhomogeneity in the exciton transition energy due to the size distribution of the quantum dots. The dephasing processes revealed by the 2PE are found to occur on at least two important time scales.

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U2 - 10.1007/978-3-642-59319-2_115

DO - 10.1007/978-3-642-59319-2_115

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VL - 71

SP - 371

EP - 373

JO - Springer Series in Chemical Physics

JF - Springer Series in Chemical Physics

ER -

Coulomb correlations, spectral line shapes, and size distributions of CdSe nanocrystals

Abstract

All Science Journal Classification (ASJC) codes

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