Abstract
The High Dimensional Model Representation (HDMR) technique is a procedure for efficiently representing high-dimensional functions. A practical form of the technique, RS-HDMR, is based on randomly sampling the overall function and utilizing orthonormal polynomial expansions. The determination of expansion coefficients employs Monte Carlo integration, which controls the accuracy of RS-HDMR expansions. In this article, a correlation method is used to reduce the Monte Carlo integration error. The determination of the expansion coefficients becomes an iteration procedure, and the resultant RS-HDMR expansion has much better accuracy than that achieved by direct Monte Carlo integration. For an illustration in four dimensions a few hundred random samples are sufficient to construct an RS-HDMR expansion by the correlation method with an accuracy comparable to that obtained by direct Monte Carlo integration with thousands of samples.
Original language | English (US) |
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Pages (from-to) | 277-283 |
Number of pages | 7 |
Journal | Journal of Computational Chemistry |
Volume | 24 |
Issue number | 3 |
DOIs | |
State | Published - Feb 2003 |
All Science Journal Classification (ASJC) codes
- General Chemistry
- Computational Mathematics
Keywords
- Atmospheric chemistry
- Correlation method with Monte Carlo integration
- HDMR
- High dimensional systems
- Random sampling