Control of two-dimensional excitonic light emission via photonic crystal

Sanfeng Wu, Sonia Buckley, Aaron M. Jones, Jason S. Ross, Nirmal J. Ghimire, Jiaqiang Yan, David G. Mandrus, Wang Yao, Fariba Hatami, Jelena Vučković, Arka Majumdar, Xiaodong Xu

Research output: Contribution to journalArticle

117 Scopus citations

Abstract

Monolayers of transition metal dichalcogenides (TMDCs) have emerged as new optoelectronic materials in the two dimensional (2D) limit, exhibiting rich spinvalley interplays, tunable excitonic effects, and strong light-matter interactions. An essential yet undeveloped ingredient for many photonic applications is the manipulation of its light emission. Here we demonstrate the control of excitonic light emission from monolayer tungsten diselenide (WSe2) in an integrated photonic structure, achieved by transferring one monolayer onto a photonic crystal (PhC) with a cavity. In addition to the observation of an effectively coupled cavity-mode emission, the suspension effects on PhC not only result in a greatly enhanced (∼60 times) photoluminescence but also strongly pattern the emission in the subwavelength spatial scale, contrasting on and off the holes. Such an effect leads to a significant diffraction grating effect, which allows us to redistribute the emitted photons both polarly and azimuthally in the far field through designing PhC structures, as revealed by momentum-resolved microscopy. A 2D optical antenna is thus constructed. Our work suggests a new way of manipulating photons in hybrid 2D photonics, important for future energy efficient optoelectronics and 2D nano-lasers.

Original languageEnglish (US)
Article number011001
Journal2D Materials
Volume1
Issue number1
DOIs
StatePublished - Jun 1 2014
Externally publishedYes

All Science Journal Classification (ASJC) codes

  • Chemistry(all)
  • Materials Science(all)
  • Condensed Matter Physics
  • Mechanics of Materials
  • Mechanical Engineering

Keywords

  • 2D semiconductor
  • Excitonic light emission
  • Optical antenna
  • Photonic crystal
  • Transition metal dichalcogenides

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  • Cite this

    Wu, S., Buckley, S., Jones, A. M., Ross, J. S., Ghimire, N. J., Yan, J., Mandrus, D. G., Yao, W., Hatami, F., Vučković, J., Majumdar, A., & Xu, X. (2014). Control of two-dimensional excitonic light emission via photonic crystal. 2D Materials, 1(1), [011001]. https://doi.org/10.1088/2053-1583/1/1/011001