Atomic-scale visualization of a cascade of magnetic orders in the layered antiferromagnet GdTe3

Arjun Raghavan, Marisa Romanelli, Julian May-Mann, Anuva Aishwarya, Leena Aggarwal, Anisha G. Singh, Maja D. Bachmann, Leslie M. Schoop, Eduardo Fradkin, Ian R. Fisher, Vidya Madhavan

Research output: Contribution to journalArticlepeer-review

1 Scopus citations

Abstract

GdTe3 is a layered antiferromagnet which has attracted attention due to its exceptionally high mobility, distinctive unidirectional incommensurate charge density wave (CDW), superconductivity under pressure, and a cascade of magnetic transitions between 7 and 12 K, with as yet unknown order parameters. Here, we use spin-polarized scanning tunneling microscopy to directly image the charge and magnetic orders in GdTe3. Below 7 K, we find a striped antiferromagnetic phase with twice the periodicity of the Gd lattice and perpendicular to the CDW. As we heat the sample, we discover a spin density wave with the same periodicity as the CDW between 7 and 12 K; the viability of this phase is supported by our Landau free energy model. Our work reveals the order parameters of the magnetic phases in GdTe3 and shows how the interplay between charge and spin can generate a cascade of magnetic orders.

Original languageEnglish (US)
Article number47
Journalnpj Quantum Materials
Volume9
Issue number1
DOIs
StatePublished - Dec 2024

All Science Journal Classification (ASJC) codes

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

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